Abstract

The control of ultrafast optical field is of great interest in developing ultrafast optics as well as the investigation on various light-matter interactions with ultrashort pulses. However, conventional spatial encoding approaches have only limited steerable targets usually neglecting the temporal effect, thus hindering their broad applications. Here we present a new concept for realizing ultrafast modulation of multi-target focal fields based on the facile combination of time-dependent vectorial diffraction theory with fast Fourier transform.

This is achieved by focusing femtosecond pulsed light carrying vectorial-vortex by a single objective lens under tight focusing condition. It is uncovered that the ultrafast temporal degree of freedom within a configurable temporal duration (~400 fs) plays a pivotal role in determining the rich and exotic features of the focused optical field at one time, namely, bright-dark alternation, periodic rotation, and longitudinal/transverse polarization conversion. The underlying control mechanisms have been unveiled.

Besides being of academic interest in diverse ultrafast spectral regimes, these peculiar behaviors of the space-time evolutionary beams may underpin prolific ultrafast-related applications such as multifunctional integrated optical chip, high-efficiency laser trapping, microstructure rotation, super-resolution optical microscopy, precise optical measurement, and liveness tracking.